Since the book was first published in 1991, the field of surface nonlinear optics has grown substantially to the point where an exposition of the principles of this field will prove useful to many. Thus, in this second edition, Chapter 8 addresses this area. Also, optical probes of magnetism of very thin films and multilayers are now widely used, and magneto-optic devices of increasing sophistication have appeared. Chapter 9 is thus devoted to magneto-optics, and associated nonlinear phenomena. The earlier chapter on "Chaos" appears as Chapter 10. The philosophy which underlies the first edition was also employed in the writing of the two new chapters. Irvine, CA D.L.Mills March 1998 Preface to the First Edition One intriguing aspect of physics is its dynamic and rapidly evolving nature; exciting new fields can become moribund within relatively few years, only to revive and grow again in a dramatic and explosive manner in response to new developments.

Electron Energy Loss Spectroscopy and Surface Vibrations is devoted to electron energy loss spectroscopy as a probe of the crystal surface. Electrons with energy in the range of a few electron volts sample only a few atomic layers. As they approach or exit from the crystal, they interact with the vibrational modes of the crystal surface, or possibly with other elementary excitations localized there. The energy spectrum of electrons back-reflected from the surface is thus a rich source of information on its dynamics. The book opens with a detailed analysis of the physics that controls the operation of the monochromator, which is the core of the experimental apparatus. Separate chapters follow on the interaction of electrons with vibrational modes of the surface region and with other elementary excitations in the vicinity; the lattice dynamics of clean and adsorbate-covered surfaces, with emphasis on those features of particular relevance to surface vibrational spectroscopy; and selected applications vibration spectroscopy in surface physics and chemistry.

Modern Problems in Condensed Matter Sciences, Volume I: Surface Polaritons: Electromagnetic Waves at Surfaces and Interfaces describes the basic properties of surface polaritons and the methods of generating these waves in the laboratory at frequencies of interest to condensed matter physicists. The selection first elaborates on surface phonon polaritons in dielectrics and semiconductors and surface exciton polaritons from the experimental viewpoint. Discussions focus on interface polaritons; surface vibrations in anisotropic crystals; experimental methods for the excitation and study of surface polaritons; and surface vibrations in isotropic crystals. The publication then ponders on surface electromagnetic wave propagation on metal surfaces; thermally stimulated emission of surface polaritons; and effects of the transition layer and spatial dispersion in the spectra of surface polaritons. The text takes a look at surface polaritons at metal surfaces and interfaces and resonance of transition layer excitations with surface polaritons. Topics include resonance of the film phonon with the substrate surface phonon polaritons; investigations of surface modifications in ultra-high vacuum; and use of surface plasma waves for the investigation of solid-liquid and solid-solid interfaces. The selection is a dependable reference for physicists and engineers wanting to conduct research on surface polaritons.

In recent years substantial progress has been made in the detection of surface phonons owing to considerable improvements in inelastic rare gas scattering tech niques and electron energy loss spectroscopy. With these methods it has become possible to measure surface vibrations in a wide energy range for all wave vectors in the two-dimensional Brillouin zone and thus to deduce the complete surface phonon dispersion curves. Inelastic atomic beam scattering and electron energy loss spectroscopy have started to play a role in the study of surface phonons similar to the one played by inelastic neutron scattering in the investigation of bulk phonons in the last thirty years. Detailed comparison between experimen tal results and theoretical studies of inelastic surface scattering and of surface phonons has now become feasible. It is therefore possible to test and to improve the details of interaction models which have been worked out theoretically in the last few decades. At this point we felt that a concise, coherent and self-contained guide to the rapidly growing field of surface phonons was needed.

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